Spatial variation of aerosol optical properties around the high-alpine site Jungfraujoch (3580 m a.s.l.)

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Abstract

This paper presents results of the extensive field campaign CLACE 2010 (Cloud and Aerosol Characterization Experiment) performed in summer 2010 at the Jungfraujoch (JFJ) and the Kleine Scheidegg (KLS) in the Swiss Alps. The main goal of this campaign was to investigate the vertical variability of aerosol optical properties around the JFJ and to show the consistency of the different employed measurement techniques considering explicitly the effects of relative humidity (RH) on the aerosol light scattering. Various aerosol optical and microphysical parameters were recorded using in-situ and remote sensing techniques. In-situ measurements of aerosol size distribution, light scattering, light absorption and scattering enhancement due to water uptake were performed at the JFJ at 3580 m a.s.l.. A unique set-up allowed remote sensing measurements of aerosol columnar and vertical properties from the KLS located about 1500 m below and within the line of sight to the JFJ (horizontal distance of approx. 4.5 km). In addition, two satellite retrievals from the Spinning Enhanced Visible and Infrared Imager (SEVIRI) and the Moderate Resolution Imaging Spectroradiometer (MODIS) as well as back trajectory analyses were added to the comparison to account for a wider geographical context. All in-situ and remote sensing measurements were in clear correspondence. The ambient extinction coefficient measured in situ at the JFJ agreed well with the KLS-based LIDAR (Light Detection and Ranging) retrieval at the altitude-level of the JFJ under plausible assumptions on the LIDAR ratio. However, we can show that the quality of this comparison is affected by orographic effects due to the exposed location of the JFJ on a saddle between two mountains and next to a large glacier. The local RH around the JFJ was often higher than in the optical path of the LIDAR measurement, especially when the wind originated from the south via the glacier, leading to orographic clouds which remained lower than the LIDAR beam. Furthermore, the dominance of long-range transported Saharan dust was observed in all measurements for several days, however only for a shorter time period in the in-situ measurements due to the vertical structure of the dust plume. The optical properties of the aerosol column retrieved from SEVIRI and MODIS showed the same magnitude and a similar temporal evolution as the measurements at the KLS and the JFJ. Remaining differences are attributed to the complex terrain and simplifications in the aerosol retrieval scheme in general. © 2012 Author(s).

Figures

  • Fig. 1. Set-up and measurement geometry during the CLACE 2010 campaign performed at the Jungfraujoch and the Kleine Scheidegg, Switzerland (red bullet on left map).
  • Fig. 2. FLEXTRA air mass trajectories (5-day backward calculations with the Jungfraujoch (JFJ) as endpoint) for the intensive observation period (3–18 July 2010). The color code denotes the specific aerosol parameter measured at the time the air parcel arrived at the site: (a) Ångström exponent of the dry scattering coefficient; (b) Ångström exponent of the dry single scattering albedo (Saharan dust index); (c) scattering enhancement factor at 85% relative humidity; (d) mean surface diameter; (e) scattering coefficient (dry); (f) aerosol optical depth measured from the Kleine Scheidegg by FUBISS-ASA2. Grey lines are trajectories without data (e.g. in cloudy situations or when measurements are below detection limit or during night-time).
  • Fig. 3. Calculated vs. measured aerosol light scattering coefficient (dry, at λ= 550 nm and a refractive index for the OPC correction of mOPC = 1.5+ 0.05i as an example). The color code denotes the Ångström exponent of the single scattering albedo αω0 , which is used to identify mineral dust at Jungfraujoch (also called Saharan dust index). Data affected by mineral dust (negative values of αω0 ) and non-affected data points (positive values of αω0 ) are fitted separately with a linear least squares regression (solid lines). The black dashed curve represents the 1:1 line.
  • Fig. 4. Example profiles of the aerosol extinction coefficient measured by the LIDAR (solid lines) at different assumed LIDAR ratios (LR) from the Kleine Scheidegg (all at λ= 355 nm). The corresponding dry and ambient extinction coefficients measured at Jungfraujoch are shown as red and blue bullet points, respectively. The webcam pictures in the upper panel are recorded at the same time (from the Kleine Scheidegg with view towards the Jungfraujoch station, see red circle). In the last example (14 July 2010) the LIDAR was measuring with a zenith angle of 60◦, missing the local cloud at the station.
  • Fig. 5. (a) Time series of the aerosol extinction coefficient (at λ= 355 nm) measured in-situ at Jungfraujoch (JFJ) (red bullets: dry, colored squares: at ambient RH indicated in the color bar) and by the LIDAR at the altitude of the JFJ (Point C and D in Fig. 1) by assuming different LIDAR ratios (see legend). (b) Ambient temperature at the JFJ (dark blue bullets) and retrieved from radiometer measurements from the Kleine Scheidegg (KLS) here at the height of the JFJ (light blue bullets). (c) Ambient relative humidity at the JFJ (dark blue bullets) and retrieved from radiometer measurements from the KLS at the height of the JFJ (light blue bullets) using the measured dew point temperature of the JFJ and the Magnus formula. (d) Wind direction measured at the JFJ. (e) The aerosol optical depth (AOD) retrieved from the LIDAR at different LIDAR ratios and measured by the Sun photometers FUBISS-ASA1 (magenta crosses) and FUBISS-ASA2 (cyan crosses). The LIDAR was operating with two different zenith angles (10◦ and 60◦, see arrows).
  • Fig. 6. Comparison of the aerosol extinction coefficient retrieved from the LIDAR measurements and in-situ measurements. The measurements from the Jungfraujoch station (at 3580 m a.s.l.) were brought to ambient conditions (solid lines) and are compared to the LIDAR measurements at different heights (100 m averages). The corresponding dry in-situ measurements (dashed lines) are shown as well. (a) Correlation coefficient for LR= 75 sr where the data is categorized by the ambient relative humidity RH (see legend above, number of points is given in brackets), (b and c) Slope and intercept of a weighted linear least squares fit for the same categorization as in panel (a). (d) Correlation coefficient for all measurements and different LR with RHamb < 80 %, (e and f) Slope and intercept for the same group of points as in panel (d).
  • Fig. 7. A strong Saharan dust event was observed by different in-situ and remote sensing instruments. (a–c) are in-situ measurements at the Jungfraujoch station. (a) Dry scattering (green line) and absorption coefficient (orange line); (b) the Ångström exponent of the single scattering albedo (Saharan dust index); (c) normalized surface size distribution measured by the SMPS and OPC (see color code), the mean surface area is shown as well (magenta line); (d) range corrected signal (RCS) of the ceilometer; (e) depolarization ratio measured by the LIDAR. Ceilometer and LIDAR measured from the Kleine Scheidegg. Horizontal magenta line: altitude of the Jungfraujoch at 3580 m a.s.l.
  • Fig. 8. Maps of daily averaged aerosol optical depth (AOD) retrieved from SEVIRI measurements for the time period of the Saharan dust event (8–11 July 2010) over Switzerland and neighboring countries. White areas are cloud and/or snow covered areas. The magenta cross denotes the location of the JFJ/KLS.

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APA

Zieger, P., Kienast-Sjögren, E., Starace, M., Von Bismarck, J., Bukowiecki, N., Baltensperger, U., … Weingartner, E. (2012). Spatial variation of aerosol optical properties around the high-alpine site Jungfraujoch (3580 m a.s.l.). Atmospheric Chemistry and Physics, 12(15), 7231–7249. https://doi.org/10.5194/acp-12-7231-2012

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